My favorites:
Griffith (Berserk)
Lamhirh (Seikai no Monshou)
Lelouch (Code Geass)
Yagami Light (Death Note)
Kotomine Kirei (FSN)
Komachi Tsugumi (Ever17)
Maou (G-senjyou no Maou)
Okabe Rintarou (Steins;Gate)
Senjougahara Hitagi (Bakemonogatari)
Takayashiki Aoba (Kazoku Keikaku)
Others I loved:
Abriel Nei Lamsar Larth Balkei Dusanyu (Seikai no Monshou)
Airs Blue (Infinite Ryvius)
Aoshi Shinomori (Rurouni Kenshin)
Count of Monte Cristo (Gankutsuou)
Dii (Utawarerumono)
Hakuoro (Utawarerumono)
Harry McDowell (Gungrave)
Houzuki Totsuan (Sharin no Kuni)
Ikari Gendo (Neon Genesis Evangelion)
Kazato Yoru (Kono Oozora ni Tsubasa wo Hirogete)
Kirijou Mitsuru (Persona 3)
Makise Kurisu (Steins;Gate)
Near (Death Note)
Nikaidou Reika (Akatsuki no Goei)
Nishi Masahito (Extravaganza)
Saitoh Hajime (Rurouni Kenshin)
Tokido Saya (Little Busters!)
Others I liked:
Ange (Umineko)
Akiba Rika (Hanbun no Tsuki ga Noboru Sora)
Alfred Arrowsmith (Bullet Butlers)
Ao (Shinigami to Shoujo)
Ari Ruruliant Houtsuki (Sharin no Kuni fan disc)
Caster (FSN)
Darth Revan (Star Wars: Knights of the Old Republic)
Death Knight Arthas Menethil (Warcraft III)
Dhaos (Tales of Phantasia)
Edwin (Baldur’s Gate)
Emiya Kiritsugu (FSN)
Eukleia (Genrin no Kishogun)
Friday Monday (Madlax)
Haryuu Claude (Oretachi ni Tsubasa ha Nai)
Hondo Sayaka (Saihate no Ima)
Illidan Stormrage (Warcraft III)
Inspector Lunge (Monster)
Kasai Kyouko (MinDeaD BlooD)
Katsuragi Yayoi (Ef -burst error-)
Keneeshu Wef Stumal Kipeil (Seikai no Monshou)
Kuonji Miyu (Kimi ga Aruji de, Ore ha shitsuji de)
Kuroro Lucifer (Hunter x Hunter)
Kyuubei (Madoka Magica)
Leon Oswald (Kaleido Star)
Lezard Valeth (Valkyrie Profile)
Liquid Snake (Metal Gear Solid)
Lucifer (Shin Megami Tensei: Nocturne)
Medicine Seller (Mononoke)
Oskar von Ruenthal (Legend of Galactic Heroes)
Paul von Oberstein (Legend of Galactic Heroes)
Raww Le Klueze (Gundam Seed)
Rito (Concert Note)
Saiyonji Akira (Himawari)
Sakurazuka Seishirou (X TV)
Sakurakouji Luna (Tsuki ni Yorisou, Otome no Sahou)
Sanzenin Nagi (Hayate no Gotoku)
Selma Fortenmayer (Bullet Butlers)
Sorimachi Ichizou (Muramasa)
Tachibana Reika (BALDR FORCE)
Takano Miyo (Higurashi)
Takaya (Persona 3)
Thage (Eternal Poison)
The M (Shikkoku no Sharnoth)
Vandelesca Grants (Tales of Abyss)
Vester (Growlanser IV)
Yoshito Kikuchi (Great Teacher Onizuka)
Visual novel & other stuff impressions 
Hello,
I disagree with some of your typings, I think Okabe of S;G is an ENTP and not an INTJ, because he loves to explore possibilites just for the sake of it, not for practical reasons (which is a sign of Ne dominance). You can see how he’s different from Makise who is the real INTJ here.
I also think Griffith is ENTJ, I find him really similar to Reinhard from Gineiden, he puts too much emphasizes on action and he’s simply too charismatic to be INTJ, and INTJ prefers to stay in the background (like Lelouch), and ENTJ likes to lead frontly (like Reinhard from Gineiden, or Reinhard from Dies Irae).
And to conclude, I think Ange is an ISFP and not an INTJ, because she has nothing really strategic like an INTJ, and she almost always let her emotions guide her. Her reaction to her bullying has nothing INTJ, she just ler herself dig into despair (Fi dominance), when an INTJ would have tried to planificate something to take revenge.
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